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Influence of palladium on the unidirectional anisotropy field in NiMn disordered systems

Identifieur interne : 000448 ( France/Analysis ); précédent : 000447; suivant : 000449

Influence of palladium on the unidirectional anisotropy field in NiMn disordered systems

Auteurs : S. Hadjoudj [France] ; S. Senoussi [France] ; M. F. Mosbah [Algérie] ; Y. Oner [Turquie]

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RBID : Pascal:98-0046144

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English descriptors

Abstract

Copyright (c) 1997 Elsevier Science B.V. All rights reserved. We have carried out AC susceptibility, hysteresis cycle and torque measurements on (Ni76-xPdx)Mn24, with 0≤x≤5, bulk alloys in the temperature and field ranges of 4.2-260 K and 0-20 kG, respectively. The AC susceptibility curves, χ′(T), present a maximum at the same freezing temperature, Tg, as the isoelectronic alloy Ni76Mn24. These alloys exhibit also the same Curie temperature, Tc, and the same saturated magnetization, Ms. However, both the unidirectional anisotropy field, Ha, and the coercivity field, Hc, increase considerably with the palladium content. For instance, Ha is 1.5 times larger for (Ni74Pd2)Mn24 than for Ni76Mn24. The torque measurements give approximately the same Ha at 4.2 K as the hysteresis cycle. We conclude that Pd impurities enhance unidirectional anisotropy but have practically no effect on Tc, Tg and Ms. This is ascribed to the greater spin-orbit coupling of palladium.


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<title xml:lang="en" level="a">Influence of palladium on the unidirectional anisotropy field in NiMn disordered systems</title>
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<title level="j" type="main">Journal of magnetism and magnetic materials</title>
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<term>Doped materials</term>
<term>Experimental study</term>
<term>Magnetic anisotropy</term>
<term>Magnetic hysteresis</term>
<term>Magnetic susceptibility</term>
<term>Magnetization</term>
<term>Manganese alloys</term>
<term>Nickel alloys</term>
<term>Palladium additions</term>
<term>Quantity ratio</term>
<term>Temperature dependence</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr">
<term>Etude expérimentale</term>
<term>Susceptibilité magnétique</term>
<term>Hystérésis magnétique</term>
<term>Effet concentration</term>
<term>Dépendance température</term>
<term>Point Curie</term>
<term>Aimantation</term>
<term>Force coercitive</term>
<term>Matériau dopé</term>
<term>Addition palladium</term>
<term>Système désordonné</term>
<term>Anisotropie magnétique</term>
<term>Nickel alliage</term>
<term>Manganèse alliage</term>
<term>Alliage binaire</term>
<term>7530G</term>
<term>7560</term>
<term>Alliage MnNi:Pd</term>
<term>Mn Ni</term>
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<div type="abstract" xml:lang="en">Copyright (c) 1997 Elsevier Science B.V. All rights reserved. We have carried out AC susceptibility, hysteresis cycle and torque measurements on (Ni
<sub>76-x</sub>
Pd
<sub>x</sub>
)Mn
<sub>24</sub>
, with 0≤x≤5, bulk alloys in the temperature and field ranges of 4.2-260 K and 0-20 kG, respectively. The AC susceptibility curves, χ′(T), present a maximum at the same freezing temperature, T
<sub>g</sub>
, as the isoelectronic alloy Ni
<sub>76</sub>
Mn
<sub>24</sub>
. These alloys exhibit also the same Curie temperature, T
<sub>c</sub>
, and the same saturated magnetization, M
<sub>s</sub>
. However, both the unidirectional anisotropy field, H
<sub>a</sub>
, and the coercivity field, H
<sub>c</sub>
, increase considerably with the palladium content. For instance, H
<sub>a</sub>
is 1.5 times larger for (Ni
<sub>74</sub>
Pd
<sub>2</sub>
)Mn
<sub>24</sub>
than for Ni
<sub>76</sub>
Mn
<sub>24</sub>
. The torque measurements give approximately the same H
<sub>a</sub>
at 4.2 K as the hysteresis cycle. We conclude that Pd impurities enhance unidirectional anisotropy but have practically no effect on T
<sub>c</sub>
, T
<sub>g</sub>
and M
<sub>s</sub>
. This is ascribed to the greater spin-orbit coupling of palladium.</div>
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